Researchers at U-M have achieved a
long-sought-after optics phenomenon that could
lead to more efficient and flexible lasers for
telecommunications and quantum computing
applications, among other uses.
The
researchers demonstrated polariton lasing for
the first time in an organic semiconductor
material at room temperature. Their results are
published in the June issue of Nature Photonics.
An organic material primarily contains
carbon, and sometimes can have biological
origin. This is in contrast to inorganic
semiconductors such as silicon or gallium
arsenide commonly found in modern electronic
circuitry.
A polariton is not exactly a particle, but it
behaves as if it were. It is a "coupled quantum
mechanical state" between an excited molecule
and a photon, or particle of light.
"You can think about it as two pendulums side
by side tied together with a spring. They have
to work together," says Stephen Forrest,
principal investigator. Forrest is the
William
Gould Dow Collegiate Professor of Electrical
Engineering, a professor in the Department
of Physics and the university's vice president
for research.
"This is a potential route to a whole bunch
of new phenomena for new applications," Forrest
says. "People have been trying to do this for
about a decade - to see polariton lasing at room
temperature. In my lab, my student Stephane Kena-Cohen
took five years to succeed in this discovery. He
had to figure out new ways to grow crystalline
organic materials between highly reflective
mirrors, and then to do the complicated
measurements with optical pulses shorter than
one-trillionth of a second."
The team is working toward building organic
lasers that, like many inorganic lasers today,
can be excited with electricity rather than
light. So-called electrically pumped lasers are
more efficient and useful than their optically
pumped counterparts. But so far, organic
semiconductors have been too fragile to survive
exposure to the amount of electrical current
necessary to get them to operate as lasers.
"We're looking at polaritons as a way to do
electrical pumping of organic semiconductors at
extremely low currents," Forrest says. "We still
optically pumped the sample in this experiment,
and the next step is to find better materials
and higher quality optical cavities in order to
eventually electrically pump the material into
lasing."
Compared to inorganic materials, organic
semiconductors offer a wider range of properties
and are easier for chemists to tailor for
specific purposes. Organics have untapped
potential in telecommunications and computing,
Forrest says.
The paper is "Room-temperature polariton
lasing in an organic single-crystal microcavity."
Forrest also is a professor in the Department of
Materials Science and Engineering. His co-author
is Stepane Kena-Cohen, a graduate student at
Princeton University.
The work was conducted at the U-M Lurie
Nanofabrication Facility. It is funded by
Universal Display Corp. (UCD) and the Air Force
Office of Scientific Research. The technology is
being licensed to UCD, a company in which
Forrest is a founder and member of the
scientific advisory board.